Modeling Polonium-212 Alpha Half-life

The incredible range of alpha decay half-lives can be modeled with quantum mechanical tunneling. The illustration represents the barrier faced by an alpha particle in polonium-212, which emits an 8.78 MeV alpha particle with a half-life of 0.3 microseconds. The following characteristics of the nuclear environment can be calculated from a basic model of the nucleus:

Separation of centers of alpha and nucleus at edge of barrier
9.1 fm
Height of barrier
26.4 MeV
Radius at which barrier drops to alpha energy
26.9 fm
Width of barrier seen by alpha
17.9 fm
Alpha's frequency of hitting the barrier
1.1 x 10^21/s
Details of calculationDifferent isotopes

The shape of the barrier must obviously be taken into account since it drops rapidly. But it is instructive to calculate the half-life for a rectangular barrier of that height and width. Using the barrier penetration calculation gives a half-life of 1.5 x 10^7 seconds, about 13 orders of magnitude longer than the observed half-life. This gives some insight into the large range of alpha half-lives; the tunneling probability depends very strongly on the nature of the barrier. The probability depends exponentially on the height and width, and in this case the height is dropping like 1/r with distance from the nucleus.

A better tunneling probability can be obtained by breaking the barrier into segments and multiplying the successive tunneling probabilities according to the basic rules for combining probabilities. The calculated tunneling probabilities for the segments are shown in the table.

Segment height
Probability
of tunneling
21.9
1.20 x10^-5
16.4
1.74 x 10^-4
13.2
1.43 x 10^-3
11.0
.98 x 10^-2
9.4
.85 x 10^-1
Product of
probabilities
2.47 x 10^-15
Details of calculation

When this tunneling probability is used to calculate the half-life, a value of 0.25 microseconds is obtained. This is surprisingly close to the measured value of 0.3 microseconds, considering that an incorrect barrier can take you off many orders of magnitude. It should be admitted that the same calculation for other nuclei does not yield such close agreement, but this example shows that the observed half-lives are within the range which can be calculated from quantum mechanical tunneling.

Index

Alpha Decay Concepts

References
Rohlf
Sec 7-4

Eisberg & Resnick
Sec 16-2
 
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